adverb
with a scraping/scratching sound
Describes a sharp, grating sound like scraping a hard surface or scratching.
猫が壁をガリッと引っかいた。
The cat scratched the wall with a scraping sound.
adverb
with a crunching sound (while eating)
Specifically for the sound of biting into something hard and crunchy, like a cracker or hard candy.
せんべいをガリッとかじった。
I bit into the rice cracker with a crunch.